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Go to tml’s local files
(If you installed via steam right click it and go to local files)
Find tmodloaderstart
Run it as administrator
Tag: controlledfolderaccess (Owner: hellcatftw#0000)
Follow the instructions here to disable controlled folder access or to add an exception for tModLoader:
https://github.com/tModLoader/tModLoader/wiki/Basic-tModLoader-Usage-FAQ#controlled-folder-access
GitHub
Basic tModLoader Usage FAQ
A mod to make and play Terraria mods. Supports Terraria 1.4 (and earlier) installations - tModLoader/tModLoader